You can also create the square using different fills by using selections and filling the result with gradients or patterns or other images et and then define the brush. You can also add effects to the square such as blurs or motion blurs or use free plugins such as the (google) Nik plugins to modify the square in 1000s of ways and then define the brush.Select the rectangle tool in the toolbar. As you're looking to create rectangular or square brushes in Photoshop, you can try following the steps mentioned below and let us know if that helps:
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